Although any soul gem can be used to capture a soul, the larger the soul, the larger the soul gem needed.
Acquire a soul gem - the types of soul gem are petty, lesser, common, greater, grand and black. As an alternative, the sword Umbra (part of the Clavicus Vile Daedric Quest), has a soul trap effect on strike, as do several other magical weapons. The longer the duration of the Soul Trap spell, the better, as you will have a longer time to capture the soul. 
You will need to have a Mysticism skill of at least 25 to use the most basic Soul Trap spell, although you can be of any level to use Soul Trap scrolls or a weapon with a Soul Trap enchantment on it.
Purchase a Soul Trap spell or scroll from any Mage's Guild hall across Cyrodiil or from another trader dealing in Soul Trap spells - you cannot capture a soul without one.
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